The attempt was one potato better than his 2004 world record of shooting eight spuds in three minutes.
"Part of the test is firing the potatoes through a tennis racket, to quantify the velocity," he said.
"A good musketeer could fire three shots a minute, which included loading, firing and cleaning the gun."
The potatoes reached speeds of up to 320km/h in the demonstration, which has still to be ratified by Guinness World Records.
Two justices of the peace, two timers and two video cameras were required to verify the feat.
The Plymouth-born educator has an international reputation for his dramatic science shows and tours the world startling and fascinating children and adults.
"Science can be dull, or it can be fascinating. It's about the delivery and talking about stuff people are interested in," he said.
"It's all about getting the 'wow' moment. Because when you get the 'wow' you get the 'why?"'
Fast facts
• 161.3km/h - Fastest cricket ball bowled (by Pakistani Shoaib Akhtar, 2003).
• 263.4km/h - Fastest tennis ball served (by Australian Samuel Groth, 2012).
• 320km/h - A potato bazooka.
• 328km/h - Fastest recorded golf ball shot.
• 720km/h - Speed of an average .22 calibre bullet.
• 1224.7km/h - Speed of sound in standard atmosphere.